New CE-TAS Paper

With the Levine group, we have posted a new paper about simulating transient absorption spectroscopy from first principles.

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Non-thermal Pseudospin Dynamics in Graphene

We have posted a new paper regarding imaging pseudospin dynamics in graphene. Working at the low excitation fluences enabled by our unique tr-ARPES instrument, we are able to vary the relative importance of electron-electron and electron-phonon scattering on the dynamics and also momentum-resolve the nascent photoexcited electrons before they relax. These are very challenging measurements due the very short carrier lifetimes in graphene and the need to resolve fine momentum-space features of the distributions.

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Myles Silfies Completes Ph. D.

Myles Silfies has successfully defended his dissertation and completed his Ph. D. Many thanks to committee members Cyrus Dreyer, Chris Johnson, and A. J. Fleisher for serving on Myles’ committee. Also thanks to Tom Weinacht (pictured at left) for helping liberate the champagne.

Myles will be working on putting frequency combs in space for Space Dynamics Laboratory in Albuquerque, NM.

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Alice Kunin featured on Princeton Chemistry Webpage

Allison lab postdoc Alice Kunin will start as an assistant professor at Princeton in Jan. 2024 where she will continue to develop advanced photoelectron spectroscopy techniques. Princeton has made a news post with more details.

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Allison Lab Research Featured in DOE Science Highlight

Our work resolving valley polarization dynamics in monolayer WS2 is now featured as a DOE office of Science Highlight.

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Ultrafast internal conversion and photochromism in gas-phase salicylideneaniline

We have posted a new paper regarding the ultrafast dynamics salicylideneanaline, combining CE-TAS measurements with ab initio theory from the Levine group.

https://arxiv.org/abs/2306.05645

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Sergii’s Farewell Dinner

Sergii Chernov is leaving us soon to start a new position at PETRA III. It was great to get the whole group together, with both new students and seasoned veterans, for an evening out.

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MRI Development Grant

In collaboration with the Liu group and the Laser Teaching Center at Stony Brook University, we will begin an exciting new five-year project to develop high-power frequency combs covering a wide swath of the electromagnetic spectrum, from the THz to the soft x-ray. The project is funded by the the Major Research Instrumentation (MRI) program of the National Science Foundation. The official announcement from NSF can be found here.

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Rotationally-resolved 2DIR spectroscopy

Using the multi-comb ideas presented in our previous paper on cavity-enhanced 2DIR spectroscopy, and major recent advances in mid-IR and long-wave IR frequency combs, high-resolution 2DIR spectroscopy of gasses is poised to become a powerful method for multi-species trace gas analysis. In two articles posted today, we present a comprehensive theoretical treatment of rotationally-resolved 2DIR (RR2DIR) spectroscopy and several new polarization conditions that can be used to bring clarity to RR2DIR spectra.

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Momentum-Resolved Exciton Coupling in Monolayer WS2

We have now posted a paper regarding our results from time-resolved ARPES studies in monolayer tungsten disulfide:

https://arxiv.org/abs/2203.02419

The momentum-space images recorded via time-of-flight momentum microscopy, like the one shown at left,  enable detailed examination of the momentum and energy dependence of coupling between exciton states across the Brillouin zone.

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